Source code for nanotools.energy

# -*- coding: utf-8 -*-
"""This module defines the ``Energy`` class."""

from ase.atoms import Atoms
from attr import field
from pint import Quantity
from nanotools.base import Base
from nanotools.system import System
from nanotools.utils import to_quantity
import attr
import numpy as np


def converter_energy(x):
    return to_quantity(x, "eV")


def converter_forces(x):
    return to_quantity(x, "eV / angstrom", shape=(-1, 3))


def converter_stress(x):
    return to_quantity(x, "eV / angstrom ** 3", shape=(3, 3))


[docs] @attr.s(auto_detect=True, eq=False) class Energy(Base): """``Energy`` class. The ``Energy`` class stores energy data. It is typically empty before a calculation. It gets overwritten during a calculation. Attributes: esr: esr is the short-range energy. Example:: esr = energy.esr ebs: ebs is the band structure energy. Example:: ebs = energy.ebs edh: edh is the delta Hartree energy. Example:: edh = energy.edh efermi: efermi is the Fermi energy. Example:: efermi = energy.efermi etot: etot is the total energy. Example:: etot = energy.etot evxc: evxc is the exchange-correlation potential energy. Example:: evxc = energy.evxc exc: exc is the exchange-correlation energy. Example:: exc = energy.exc eigenvalues: eigenvalues is a three-dimensional array containing the Kohn-Sham energies (the eigenvalues of the Kohn-Sham equation). The dimensions are the following: bands, k-point, spin. Example:: eigenvalues = energy.eigenvalues forces: forces is a two-dimensional array containing the atomic forces (as calculated by the Hellman-Feynman theorem). Example:: forces = energy.forces forces_return: If True, the forces are computed and written to energy.forces. They are not computed otherwise. Example:: energy.forces_return = True stress: stress is a two-dimensional array containing the stress tensor (as calculated by the Hellman-Feynman theorem). Example:: stress = energy.stress stress_return: If True, the stress tensor is computed and written to energy.stress. It is not computed otherwise. Example:: energy.stress_return = True edftd3: Grimme's DFT-D3 energy. It is evaluated with ASE's `DFTD3 calculator <https://wiki.fysik.dtu.dk/ase/ase/calculators/dftd3.html>`_. For additional details on the methods, please visit the Mulliken Center's `website <https://www.chemie.uni-bonn.de/pctc/mulliken-center/software/dft-d3/>`_. frc_dftd3: Grimme's DFT-D3 forces. stress_dftd3: Grimme's DFT-D3 stress. include_dftd3: Grimme's DFT-D3 switch. If True, include D3 dispersion corrections in energy, forces and stress. Do nothing otherwise. """ esr: Quantity = field( default=None, converter=attr.converters.optional(converter_energy), validator=attr.validators.optional(attr.validators.instance_of(Quantity)), ) ebg: Quantity = field( default=None, converter=attr.converters.optional(converter_energy), validator=attr.validators.optional(attr.validators.instance_of(Quantity)), ) ebs: Quantity = field( default=None, converter=attr.converters.optional(converter_energy), validator=attr.validators.optional(attr.validators.instance_of(Quantity)), ) edh: Quantity = field( default=None, converter=attr.converters.optional(converter_energy), validator=attr.validators.optional(attr.validators.instance_of(Quantity)), ) exc: Quantity = field( default=None, converter=attr.converters.optional(converter_energy), validator=attr.validators.optional(attr.validators.instance_of(Quantity)), ) evxc: Quantity = field( default=None, converter=attr.converters.optional(converter_energy), validator=attr.validators.optional(attr.validators.instance_of(Quantity)), ) etot: Quantity = field( default=None, converter=attr.converters.optional(converter_energy), validator=attr.validators.optional(attr.validators.instance_of(Quantity)), ) efermi: Quantity = field( default=None, converter=attr.converters.optional(converter_energy), validator=attr.validators.optional(attr.validators.instance_of(Quantity)), ) eigenvalues: Quantity = field( default=None, converter=attr.converters.optional(converter_energy), validator=attr.validators.optional(attr.validators.instance_of(Quantity)), ) efree: Quantity = field( default=None, converter=attr.converters.optional(converter_energy), validator=attr.validators.optional(attr.validators.instance_of(Quantity)), ) entropy: Quantity = field( default=None, converter=attr.converters.optional(converter_energy), validator=attr.validators.optional(attr.validators.instance_of(Quantity)), ) forces: Quantity = field( default=None, converter=attr.converters.optional(converter_forces), validator=attr.validators.optional(attr.validators.instance_of(Quantity)), ) forces_return: bool = field( default=False, converter=bool, validator=attr.validators.instance_of(bool), ) stress: Quantity = field( default=None, converter=attr.converters.optional(converter_stress), validator=attr.validators.optional(attr.validators.instance_of(Quantity)), ) stress_return: bool = field( default=False, converter=bool, validator=attr.validators.instance_of(bool), ) frc_t: Quantity = field( default=None, converter=attr.converters.optional(converter_forces), validator=attr.validators.optional(attr.validators.instance_of(Quantity)), ) frc_s: Quantity = field( default=None, converter=attr.converters.optional(converter_forces), validator=attr.validators.optional(attr.validators.instance_of(Quantity)), ) frc_vnl: Quantity = field( default=None, converter=attr.converters.optional(converter_forces), validator=attr.validators.optional(attr.validators.instance_of(Quantity)), ) frc_veff: Quantity = field( default=None, converter=attr.converters.optional(converter_forces), validator=attr.validators.optional(attr.validators.instance_of(Quantity)), ) frc_sr: Quantity = field( default=None, converter=attr.converters.optional(converter_forces), validator=attr.validators.optional(attr.validators.instance_of(Quantity)), ) frc_vna: Quantity = field( default=None, converter=attr.converters.optional(converter_forces), validator=attr.validators.optional(attr.validators.instance_of(Quantity)), ) frc_vdh: Quantity = field( default=None, converter=attr.converters.optional(converter_forces), validator=attr.validators.optional(attr.validators.instance_of(Quantity)), ) frc_rpc: Quantity = field( default=None, converter=attr.converters.optional(converter_forces), validator=attr.validators.optional(attr.validators.instance_of(Quantity)), ) edftd3: Quantity = field( default=None, converter=attr.converters.optional(converter_energy), validator=attr.validators.optional(attr.validators.instance_of(Quantity)), ) frc_dftd3: Quantity = field( default=None, converter=attr.converters.optional(converter_forces), validator=attr.validators.optional(attr.validators.instance_of(Quantity)), ) stress_dftd3: Quantity = field( default=None, converter=attr.converters.optional(converter_stress), validator=attr.validators.optional(attr.validators.instance_of(Quantity)), ) include_dftd3: bool = attr.ib( default=False, converter=bool, validator=attr.validators.instance_of(bool), ) dftd3_kwargs: dict = attr.ib(default=attr.Factory(dict)) def __attrs_post_init__(self): pass def __eq__(self, other): if other.__class__ is not self.__class__: return NotImplemented valid = True for at in ( "eigenvalues", # arrays of floats "forces", "stress", "esr", # floats "ebg", "ebs", "edh", "exc", "evxc", "etot", "efermi", "efree", "entropy", ): if getattr(self, at) is None: valid = valid and getattr(self, at) == getattr(other, at) else: valid = valid and np.allclose(getattr(self, at), getattr(other, at)) return valid and ( self.esr.u, self.ebg.u, self.ebs.u, self.edh.u, self.exc.u, self.evxc.u, self.etot.u, self.efermi.u, self.eigenvalues.u, self.efree.u, self.entropy.u, self.forces.u, self.forces_return, self.stress.u, self.stress_return, ) == ( other.esr.u, other.ebg.u, other.ebs.u, other.edh.u, other.exc.u, other.evxc.u, other.etot.u, other.efermi.u, other.eigenvalues.u, other.efree.u, other.entropy.u, other.forces.u, other.forces_return, other.stress.u, other.stress_return, ) def get_band_edges(self): emin = np.min(self.eigenvalues) emax = np.max(self.eigenvalues) return emin - 1, emax + 1
[docs] def get_cbm(self): """ Returns the conduction band maximum. If partially occupied bands are detected, as in metals, then the function returns ``None``. Returns: float: conduction band maximum """ if self.ismetal(): return None ev = self.eigenvalues return np.min(ev[ev > self.efermi])
[docs] def get_free_energy(self): """Returns the free energy.""" return self.efree
[docs] def get_total_energy(self): """Returns the total energy.""" return self.etot
[docs] def get_vbm(self): """ Returns the valence band maximum. If partially occupied bands are detected, as in metals, then the function returns ``None``. Returns: float: valence band maximum """ if self.ismetal(): return None ev = self.eigenvalues return np.max(ev[ev < self.efermi])
[docs] def ismetal(self): """Determines whether the band structure is metallic. The band structure is metallic if some bands are partially filled at zero temperature. The function determines band occupancy based on the Fermi level. Note that the Fermi level may cut the VBM or CBM of semiconductors or insulators depending on the occupation scheme and k-sampling mesh. Returns: bool: True if metallic, False otherwise """ issemi = np.all(self.eigenvalues < self.efermi, axis=(1, 2)) issemi = np.logical_or( issemi, np.all(self.eigenvalues > self.efermi, axis=(1, 2)) ) return not np.all(issemi)
[docs] def set_stress_return(self, stress_return): """Sets stress_return attribute. If stress_return is True, then forces_return is also set to True. Args: stress_return (bool): stress_return value """ if not isinstance(stress_return, bool): raise Exception( f"Invalid class {stress_return.__class__} for arg stress_return." ) self.stress_return = stress_return if self.stress_return: self.forces_return = True
def set_dftd3_energy(self, atoms, include_dftd3=True, **kwargs): from ase.calculators.dftd3 import DFTD3 from ase.atoms import Atoms if isinstance(atoms, System): atoms = atoms.to_ase_atoms() elif isinstance(atoms, Atoms): pass else: raise Exception("Argument atoms must be of class System or ASE Atoms.") self.dftd3_kwargs.update(kwargs) self.include_dftd3 = include_dftd3 d3 = DFTD3(**self.dftd3_kwargs) atoms.calc = d3 self.edftd3 = to_quantity(atoms.get_potential_energy(), "eV") self.frc_dftd3 = to_quantity(atoms.get_forces(), "eV / angstrom", shape=(-1, 3)) self.stress_dftd3 = to_quantity( atoms.get_stress(voigt=False), "eV / angstrom ** 3", shape=(3, 3) ) self._update_energy_forces_stress() set_dftd3_forces = set_dftd3_stress = set_dftd3_energy def _update_energy_forces_stress(self): if not self.include_dftd3: return ats = ["etot", "efree", "forces", "stress"] d3s = ["edftd3", "edftd3", "frc_dftd3", "stress_dftd3"] for a, d in zip(ats, d3s): frc = getattr(self, a) dfr = getattr(self, d) if frc is None: setattr(self, a, dfr) else: setattr(self, a, frc + dfr)